Artigo Acesso aberto Revisado por pares

Spin Densities in Dimesitylmethyl

1960; American Institute of Physics; Volume: 32; Issue: 5 Linguagem: Inglês

10.1063/1.1730946

ISSN

1520-9032

Autores

A. McLachlan,

Tópico(s)

Chemical Reactions and Mechanisms

Resumo

A simple valence bond calculation indicates that if the dimesitylmethyl radical were planar large unpaired spin densities would appear on the ring methyl groups giving a spectrum about 130 gauss wide. A perturbation calculation, assuming that the molecule is very twisted, gives spin densities ρ1=1.000, ρ2=—0.069, ρ3=0.054, ρ4=—0.040, ρ5=0.043 on the carbon atoms, numbered from the center outwards.

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