Radical polymerization of methacrylic acid in the presence of poly(4‐vinylpyridine) in methanol

1979; Wiley; Volume: 180; Issue: 7 Linguagem: Inglês

10.1002/macp.1979.021800712

ISSN

0025-116X

Autores

Kiyohisa Fujimori,

Tópico(s)

Polymer Science and PVC

Resumo

Abstract The rate of radical polymerization of methacrylic acid (MA) was found enhanced in the presence of poly(4‐vinylpyridine) (P4VP) of various molecular weights (M̄ η ) in methanol. The rate maximum shifted from 1 : 1 mole ratio of [P4VP]/[MA], based on the repeating units, to a larger polymer‐monomer ratio and also the rate enhancement was smaller, when P4VP of smaller M̄ η was used. The overall energy of activation was 36,1 and 60,7 kJ/mol in the presence and absence of P4VP, respectively. The M̄ η of poly(methacrylic acid) (PMA) prepared with P4VP was about 10 times larger than the M̄ η of PMA prepared without P4VP.

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