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Enhancing catalytic activity and stability for CO 2 methanation on Ni@MOF-5 via control of active species dispersion

2014; Royal Society of Chemistry; Volume: 51; Issue: 9 Linguagem: Inglês

10.1039/c4cc08733j

1364-548X

Wenlong Zhen, Bo Li, Gongxuan Lü, Jiantai Ma,

CO2 Reduction Techniques and Catalysts

A novel, highly active catalyst Ni@MOF-5 showed unexpected activity at low temperature for CO2 methanation. The characterization results indicated that Ni was uniformly and highly dispersed over MOF-5. This catalyst showed high stability and almost no deactivation in long term stability tests up to 100 h.