Multiple-scattering X alpha calculation of spectral energies involving the π and π* orbitals of C 2 H 2

1985; IOP Publishing; Volume: 18; Issue: 3 Linguagem: Inglês

10.1088/0022-3700/18/3/014

ISSN

1747-3721

Autores

J. A. Tossell,

Tópico(s)

Mass Spectrometry Techniques and Applications

Resumo

Bound-state and continuum multiple-scattering (MS) X alpha calculations on C2H2 yield values accurate to within 0.8 eV for the pi IP, the average pi to pi * excitation energy, the C 1s to pi and C 1s to pi * X-ray excitation energies, the pi to pi * C 1s shake-up satellite energy, the pi * attachment energy and the pi 4 to pi 3 sigma *2 Feshbach resonance energy. The derivative electron transmission spectrum of C2H2 is shown for the first time. Quantitative relationships between the different spectral properties are established using the transition state approach.

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