Artigo Revisado por pares

Interface segregation in copolymer blends measured by neutron reflection and secondary ion mass spectrometry

1991; Elsevier BV; Volume: 173; Issue: 1-2 Linguagem: Inglês

10.1016/0921-4526(91)90050-o

ISSN

1873-2135

Autores

T. Mansfield, Richard S. Stein, Russell J. Composto, Miriam Rafailovich, Konstantin Sokolov, S. A. Schwarz,

Tópico(s)

Nanopore and Nanochannel Transport Studies

Resumo

Abstract In polymer blends of poly(styrene-co-acrylonitrile) (SAN) differing in acrylonitrile content, the SAN with the lower acrylonitrile component enriches the vacuum-polymer and polymer-substrate interfaces. The concentration profiles determined by neutron reflection measurements yield an interfacial excess of 80 and 38 A near the surface and substrate, respectively. Using contrast matching, neutron reflection is shown to be quite sensitive to segregation near buried interfaces. Depths profiles measured by neutron reflection and secondary-ion mass spectrometry are in good qualitative agreement.

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