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Phase Control of Rotational Wave Packets and Quantum Information

2004; American Physical Society; Volume: 93; Issue: 23 Linguagem: Inglês

10.1103/physrevlett.93.233601

1092-0145

Kevin F. Lee, D. M. Villeneuve, P. B. Corkum, E. A. Shapiro,

Quantum optics and atomic interactions

Lasers can create rotational wave packets in gas-phase molecules which periodically revive as field-free, aligned distributions. We control the wave packet evolution with relatively weak laser pulses at fractional revivals which modify the phase between wave packet components. We demonstrate two phase control effects in oxygen: coherently switching revivals off and on, and doubling the revival frequency. When viewed as a quantum logic system, these effects correspond to a Hadamard and a T operation.