Artigo Revisado por pares

Synthesis of 6,5-fused bicyclic lactams as potential dipeptide β-turn mimetics

1994; Elsevier BV; Volume: 35; Issue: 24 Linguagem: Inglês

10.1016/s0040-4039(00)73120-0

ISSN

1873-3581

Autores

Rudolf Mueller, Láśzló Révész,

Tópico(s)

Synthesis and Catalytic Reactions

Resumo

The first short synthesis of the dipeptide mimetic (3S, 6S, 9S)-6-amino-5-oxoindolizidine-3-carboxylic acid 1 and its Z-protected derivative 9 is described, employing the Schoellkopf bislactim-ether methodology, followed by a highly specific intramolecular reductive amination and spontaneous lactamization. These 6,5-fused bicyclic lactams may be viewed as conformationally restricted alanyl-proline β-turn mimetics.

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