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Heavy-hole and light-hole oscillations in the coherent emission from quantum wells: Evidence for exciton-exciton correlations

1999; American Physical Society; Volume: 60; Issue: 11 Linguagem: Inglês

10.1103/physrevb.60.8267

1095-3795

Arthur L. Smirl, Martin J. Stevens, Xi Chen, O. Buccafusca,

Spectroscopy and Quantum Chemical Studies

We demonstrate the presence of strong exciton-exciton correlations in GaAs-AlGaAs multiple quantum wells by using the polarization selection rules for four-wave mixing and a test that was originally designed to distinguish between quantum beats and polarization interference. We show that, when the four-wave-mixing signal is produced by two pulses that have the same circular polarization, dynamic beating behavior is observed at the heavy-hole-light-hole frequency that provides evidence of Coulomb-induced correlations that go beyond those expected from the semiconductor Bloch equations in the Hartree-Fock approximation and beyond the local field corrections used in simple phenomenological models. Moreover, this behavior cannot be explained by invoking biexcitonic effects. We demonstrate that this dynamic excitonic coupling can be explained in terms of a competition between quantum-beat-like and polarization-interference-like behavior, and we show that such behavior can be used to place quantitative limits on the coupling strength. In addition, we use a simple phenomenological model to show that excitation-induced-dephasing can produce such correlations.