Artigo Acesso aberto

Electrochemical reactivity of biologically active quinone/hydroquinone sesquiterpenoids on glassy carbon electrodes

1987; Elsevier BV; Volume: 17; Issue: 3 Linguagem: Inglês

10.1016/0302-4598(87)80064-8

ISSN

1872-8049

Autores

Ibro Tabaković, Asima Davidović, Wernér E.G. Müller, Rudolf K. Ζahn, Dušan Sladić, Nikola Dogović, Miroslav J. Gašić,

Tópico(s)

Marine Sponges and Natural Products

Resumo

The redox reactivity of avarone and avarol, a quinone/hydroquinone couple isolated from the marine sponge Dysidea avara, was investigated by cyclic voltammetry, using a glassy carbon electrode. Both oxidation of avarol and reduction of avarone in aqueous ethanol (1:1 V/V) take place by a 2 e− process at a wide range of pH values; in acetonitrile, however, the reduction of avarone occurs as a stepwise electron transfer process. The mechanisms, as well as the scope and limitations of the method are discussed with reference to the biological activity of the two sesquiterpenoids.

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