Artigo Revisado por pares

Rate of Some Hydroxyl Radical Reactions

1970; American Institute of Physics; Volume: 52; Issue: 3 Linguagem: Inglês

10.1063/1.1673102

ISSN

1520-9032

Autores

J. E. Breen, G. Glass,

Tópico(s)

Advanced oxidation water treatment

Resumo

The rates of the following reactions of the hydroxyl radical have been measured in a fast flow system using ESR detection: OH+OH→H2O+O, OH+O→H+O2, OH→wall. The rate constants obtained were k1 = 8.4 ± 2.6 × 10−13cm3molecule−1·sec−1, k2 = 4.3 ± 1.3 × 10−11cm3molecule−1·sec−1, and k3 = 124 ± 40 sec−1. The rates of the first two reactions are compared with previous measurements. Earlier investigators have not included the third reaction in their mechanisms. In all experiments, the hydroxyl radicals were generated by means of the titration reaction H + NO2→OH + NO.

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