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Direct measurement of the upper critical field in cuprate superconductors

2014; Nature Portfolio; Volume: 5; Issue: 1 Linguagem: Inglês

10.1038/ncomms4280

2041-1723

G. Grissonnanche, O. Cyr-Choinière, F. Laliberté, S. René de Cotret, Alexandre Juneau-Fecteau, Sophie Dufour-Beauséjour, M. Delage, David LeBoeuf, J. Chang, B. J. Ramshaw, D. A. Bonn, W. N. Hardy, R. Liang, Seiji Adachi, N. E. Hussey, Baptiste Vignolle, Cyril Proust, M. Sutherland, S. Krämer, J.-H. Park, David Graf, N. Doiron-Leyraud, Louis Taillefer,

Iron-based superconductors research

In the quest to increase the critical temperature Tc of cuprate superconductors, it is essential to identify the factors that limit the strength of superconductivity. The upper critical field Hc2 is a fundamental measure of that strength, yet there is no agreement on its magnitude and doping dependence in cuprate superconductors. Here we show that the thermal conductivity can be used to directly detect Hc2 in the cuprates YBa2Cu3Oy, YBa2Cu4O8 and Tl2Ba2CuO6+δ, allowing us to map out Hc2 across the doping phase diagram. It exhibits two peaks, each located at a critical point where the Fermi surface of YBa2Cu3Oy is known to undergo a transformation. Below the higher critical point, the condensation energy, obtained directly from Hc2, suffers a sudden 20-fold collapse. This reveals that phase competition—associated with Fermi-surface reconstruction and charge-density-wave order—is a key limiting factor in the superconductivity of cuprates. The point at which a magnetic field kills superconductivity in the cuprates has been difficult to measure. Grissonnanche et al. use thermal conductivity measurements to reliably determine this field and find that it drops suddenly below some critical doping, suggesting the onset of a new competing phase.