Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy
2010; Wiley; Volume: 16; Issue: 43 Linguagem: Inglês
10.1002/chem.201001844
ISSN1521-3765
AutoresTeng He, Junhu Wang, Guotao Wu, Hyunjeong Kim, Thomas Proffen, Anan Wu, Wen Li, Tao Liu, Zhitao Xiong, Chengzhang Wu, Hailiang Chu, Jianping Guo, Tom Autrey, Tao Zhang, Ping Chen,
Tópico(s)Ammonia Synthesis and Nitrogen Reduction
ResumoChemistry – A European JournalVolume 16, Issue 43 p. 12814-12817 Communication Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy Teng He, Teng He Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorProf. Junhu Wang, Prof. Junhu Wang Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Guotao Wu, Dr. Guotao Wu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Hyunjeong Kim, Dr. Hyunjeong Kim Lujan Neutron Scattering Center, Los Alamos National Laboratory, Los Alamos, New Mexico, 87545 (USA)Search for more papers by this authorDr. Thomas Proffen, Dr. Thomas Proffen Lujan Neutron Scattering Center, Los Alamos National Laboratory, Los Alamos, New Mexico, 87545 (USA)Search for more papers by this authorDr. Anan Wu, Dr. Anan Wu State Key laboratory of Physical Chemical of Solid Surfaces, Xiamen University, YanWu Road, Xiamen, Fujian, 361005 (China)Search for more papers by this authorWen Li, Wen Li Department of Physics, National University of Singapore, 10 Kent Ridge Crescent, 117542 (Singapore)Search for more papers by this authorTao Liu, Tao Liu Institute for Synchrotron Radiation, Karlsruhe Institute of Technology, 76344 Karlsruhe (Germany)Search for more papers by this authorProf. Zhitao Xiong, Prof. Zhitao Xiong Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Chengzhang Wu, Dr. Chengzhang Wu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Hailiang Chu, Dr. Hailiang Chu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorJianping Guo, Jianping Guo Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Tom Autrey, Dr. Tom Autrey Pacific Northwest National Laboratory, Richland, WA 99352 (USA)Search for more papers by this authorProf. Tao Zhang, Prof. Tao Zhang Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorProf. Ping Chen, Prof. Ping Chen [email protected] Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this author Teng He, Teng He Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorProf. Junhu Wang, Prof. Junhu Wang Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Guotao Wu, Dr. Guotao Wu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Hyunjeong Kim, Dr. Hyunjeong Kim Lujan Neutron Scattering Center, Los Alamos National Laboratory, Los Alamos, New Mexico, 87545 (USA)Search for more papers by this authorDr. Thomas Proffen, Dr. Thomas Proffen Lujan Neutron Scattering Center, Los Alamos National Laboratory, Los Alamos, New Mexico, 87545 (USA)Search for more papers by this authorDr. Anan Wu, Dr. Anan Wu State Key laboratory of Physical Chemical of Solid Surfaces, Xiamen University, YanWu Road, Xiamen, Fujian, 361005 (China)Search for more papers by this authorWen Li, Wen Li Department of Physics, National University of Singapore, 10 Kent Ridge Crescent, 117542 (Singapore)Search for more papers by this authorTao Liu, Tao Liu Institute for Synchrotron Radiation, Karlsruhe Institute of Technology, 76344 Karlsruhe (Germany)Search for more papers by this authorProf. Zhitao Xiong, Prof. Zhitao Xiong Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Chengzhang Wu, Dr. Chengzhang Wu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Hailiang Chu, Dr. Hailiang Chu Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorJianping Guo, Jianping Guo Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorDr. Tom Autrey, Dr. Tom Autrey Pacific Northwest National Laboratory, Richland, WA 99352 (USA)Search for more papers by this authorProf. Tao Zhang, Prof. Tao Zhang Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this authorProf. Ping Chen, Prof. Ping Chen [email protected] Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86) 411-84685940Search for more papers by this author First published: 11 October 2010 https://doi.org/10.1002/chem.201001844Citations: 39Read the full textAboutPDF ToolsRequest permissionExport citationAdd to 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Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Graphical Abstract Nano-alloy: Crystalline polyaminoborane is formed upon releasing 1.0 equivalent H2 from ammonia borane at 60 °C catalyzed by a nano-FeB alloy. Our experimental results show that about 1.0 and 1.5 equiv H2 can be released at 60 and 100 °C, respectively. Supporting Information Detailed facts of importance to specialist readers are published as "Supporting Information". Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Filename Description chem_201001844_sm_miscellaneous_information.pdf463.4 KB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. References 1S. Orimo, Y. Nakamori, J. R. Eliseo, A. Züttel, C. M. 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