The Active Phase of Nickel/Ordered Ce 2 Zr 2 O x Catalysts with a Discontinuity ( x =7 – 8) in Methane Steam Reforming
2012; Wiley; Volume: 51; Issue: 37 Linguagem: Inglês
10.1002/anie.201205167
ISSN1521-3773
AutoresMizuki Tada, Shenghong Zhang, Sachin Malwadkar, Nozomu Ishiguro, Jun‐ichi Soga, Yasutaka Nagai, Keitaro Tezuka, Hideo Imoto, Shinya Otsuka‐Yao‐Matsuo, Shin‐ichi Ohkoshi, Yasuhiro Iwasawa,
Tópico(s)Catalysis and Oxidation Reactions
ResumoAngewandte Chemie International EditionVolume 51, Issue 37 p. 9361-9365 Communication The Active Phase of Nickel/Ordered Ce2Zr2Ox Catalysts with a Discontinuity (x=7–8) in Methane Steam Reforming† Dr. Mizuki Tada, Corresponding Author Dr. Mizuki Tada mtada@ims.ac.jp Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) The Graduate University of Advanced Studies (SOKENDAI), 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Mizuki Tada, Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Yasuhiro Iwasawa, The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this authorDr. Shenghong Zhang, Dr. Shenghong Zhang Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan)Search for more papers by this authorDr. Sachin Malwadkar, Dr. Sachin Malwadkar The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this authorNozomu Ishiguro, Nozomu Ishiguro Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorJun-ichi Soga, Jun-ichi Soga Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorDr. Yasutaka Nagai, Dr. Yasutaka Nagai Toyota Central R&D Labs. Inc. (Japan)Search for more papers by this authorDr. Keitaro Tezuka, Dr. Keitaro Tezuka Department of Applied Chemistry, Utsunomiya University (Japan)Search for more papers by this authorProf. Dr. Hideo Imoto, Prof. Dr. Hideo Imoto Department of Applied Chemistry, Utsunomiya University (Japan)Search for more papers by this authorProf. Dr. Shinya Otsuka-Yao-Matsuo, Prof. Dr. Shinya Otsuka-Yao-Matsuo Graduate School of Engineering, Osaka University (Japan)Search for more papers by this authorProf. Dr. Shin-ichi Ohkoshi, Prof. Dr. Shin-ichi Ohkoshi Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorProf. Dr. Yasuhiro Iwasawa, Corresponding Author Prof. Dr. Yasuhiro Iwasawa iwasawa@pc.uec.ac.jp The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan) Mizuki Tada, Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Yasuhiro Iwasawa, The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this author Dr. Mizuki Tada, Corresponding Author Dr. Mizuki Tada mtada@ims.ac.jp Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) The Graduate University of Advanced Studies (SOKENDAI), 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Mizuki Tada, Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Yasuhiro Iwasawa, The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this authorDr. Shenghong Zhang, Dr. Shenghong Zhang Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan)Search for more papers by this authorDr. Sachin Malwadkar, Dr. Sachin Malwadkar The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this authorNozomu Ishiguro, Nozomu Ishiguro Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorJun-ichi Soga, Jun-ichi Soga Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorDr. Yasutaka Nagai, Dr. Yasutaka Nagai Toyota Central R&D Labs. Inc. (Japan)Search for more papers by this authorDr. Keitaro Tezuka, Dr. Keitaro Tezuka Department of Applied Chemistry, Utsunomiya University (Japan)Search for more papers by this authorProf. Dr. Hideo Imoto, Prof. Dr. Hideo Imoto Department of Applied Chemistry, Utsunomiya University (Japan)Search for more papers by this authorProf. Dr. Shinya Otsuka-Yao-Matsuo, Prof. Dr. Shinya Otsuka-Yao-Matsuo Graduate School of Engineering, Osaka University (Japan)Search for more papers by this authorProf. Dr. Shin-ichi Ohkoshi, Prof. Dr. Shin-ichi Ohkoshi Department of Chemistry, Graduate School of Science, The University of Tokyo (Japan)Search for more papers by this authorProf. Dr. Yasuhiro Iwasawa, Corresponding Author Prof. Dr. Yasuhiro Iwasawa iwasawa@pc.uec.ac.jp The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan) Mizuki Tada, Institute for Molecular Science, 38 Nishigo-naka, Myodaiji, Okazaki, Aichi 444-8585 (Japan) Yasuhiro Iwasawa, The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)Search for more papers by this author First published: 21 August 2012 https://doi.org/10.1002/anie.201205167Citations: 29 † This work was supported by the Funding Program for Next Generation World-Leading Researchers (GR090) from the Cabinet Office, Government of Japan, a Grant-in-Aid for Scientific Research (S) (No. 18106013) from MEXT (Japan), and the Joint Studies Program of IMS (2009-2010). XAFS measurements were performed with the approval of PF-PAC (Nos. 2006G337 and 2008G188). Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onFacebookTwitterLinked InRedditWechat Abstract Breaking news: A unique discontinuous property and an active phase of Ni/ordered Ce2Zr2Ox (x=7–8) solid-solution catalysts were observed during methane steam reforming. The catalytic performance of Ni/Ce2Zr2Ox strongly depended on the phase and oxygen content of the Ce2Zr2Ox support. Citing Literature Supporting Information Detailed facts of importance to specialist readers are published as ”Supporting Information”. Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Filename Description anie_201205167_sm_miscellaneous_information.pdf1,023.8 KB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume51, Issue37September 10, 2012Pages 9361-9365 RelatedInformation
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