Artigo Revisado por pares

The wulfenite—stolzite series: centric or acentric structures?

2008; Cambridge University Press; Volume: 72; Issue: 4 Linguagem: Inglês

10.1180/minmag.2008.072.4.987

ISSN

1471-8022

Autores

L. Secco, Fabrizio Nestola, A. Dal Negro,

Tópico(s)

Polyoxometalates: Synthesis and Applications

Resumo

Abstract Three natural crystals of the wulfenite (PbMoO 4 )—stolzite (PbWO 4 ) series were investigated by single-crystal X-ray diffraction. The results indicate that the symmetry is I4 1 /a from nearly pure wulfenite to intermediate compositions, in contrast to previous work which claimed a symmetry change to 74 symmetry (acentric) for intermediate compositions compared with I4 1 /a (centric space group) for the end-members. The results reported here show that the reflections violating I4 1 /a symmetry observed in this work and in a previous study are related primarily to λ/2 effects, even if Renninger effects are not excluded. Consequently, we find that the I4 1 /a symmetry is retained throughout the wulfenite— stolzite.

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