Water Splitting by Tungsten Oxide Prepared by Atomic Layer Deposition and Decorated with an Oxygen‐Evolving Catalyst
2010; Wiley; Volume: 50; Issue: 2 Linguagem: Inglês
10.1002/anie.201004801
ISSN1521-3773
AutoresRui Liu, Yongjing Lin, Lien‐Yang Chou, Stafford W. Sheehan, Wangshu He, Fan Zhang, Harvey J. M. Hou, Dunwei Wang,
Tópico(s)Advanced Photocatalysis Techniques
ResumoAngewandte Chemie International EditionVolume 50, Issue 2 p. 499-502 Communication Water Splitting by Tungsten Oxide Prepared by Atomic Layer Deposition and Decorated with an Oxygen-Evolving Catalyst† Rui Liu, Rui Liu Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorYongjing Lin, Yongjing Lin Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorLien-Yang Chou, Lien-Yang Chou Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorStafford W. Sheehan, Stafford W. Sheehan Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorWangshu He, Wangshu He Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorFan Zhang, Fan Zhang Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorProf. Dr. Harvey J. M. Hou, Corresponding Author Prof. Dr. Harvey J. M. Hou [email protected] Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Harvey J. M. Hou, Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Dunwei Wang, Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorProf. Dr. Dunwei Wang, Corresponding Author Prof. Dr. Dunwei Wang [email protected] Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwang Harvey J. M. Hou, Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Dunwei Wang, Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this author Rui Liu, Rui Liu Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorYongjing Lin, Yongjing Lin Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorLien-Yang Chou, Lien-Yang Chou Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorStafford W. Sheehan, Stafford W. Sheehan Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorWangshu He, Wangshu He Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorFan Zhang, Fan Zhang Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/Search for more papers by this authorProf. Dr. Harvey J. M. Hou, Corresponding Author Prof. Dr. Harvey J. M. Hou [email protected] Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Harvey J. M. Hou, Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Dunwei Wang, Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this authorProf. Dr. Dunwei Wang, Corresponding Author Prof. Dr. Dunwei Wang [email protected] Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwang Harvey J. M. Hou, Department of Chemistry and Biochemistry, University of Massachusetts Dartmouth, North Dartmouth, MA 02747 (USA) http://www.faculty.umassd.edu/harveyjianmin.hou/ Dunwei Wang, Department of Chemistry, Merkert Chemistry Center, Boston College, 2609 Beacon St., Chestnut Hill, MA 02467 (USA), Fax: (+1) 617-552-2705 http://www2.bc.edu/∼dwangSearch for more papers by this author First published: 09 December 2010 https://doi.org/10.1002/anie.201004801Citations: 274 † We acknowledge financial support from Boston College and the University of Massachusetts Dartmouth, technical support from Dr. X. Liu, S. Zhou, Dr. E. Ojadi, C. Leidhold, N. Geh, and S. Cederlund. This work is partially supported by a NSF instrumentation grant (DRM 0821471) to D.W. The XPS experiments were conducted at the Materials Center at MIT. Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Graphical Abstract Heteronanostructured photoelectrodes were fabricated by atomic layer deposition of WO3 and stabilized with an Mn-based oxygen-evolving catalyst. The resulting electrode absorbs photons to create electrons and holes, the separation of which is assisted by the built-in field within the semiconductor. Electrons are collected, and holes transferred to the catalyst to split H2O into oxygen and hydrogen (see schematic). Citing Literature Supporting Information Detailed facts of importance to specialist readers are published as "Supporting Information". Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Filename Description anie_201004801_sm_miscellaneous_information.pdf2.4 MB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume50, Issue2January 10, 2011Pages 499-502 RelatedInformation
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