Revisão Revisado por pares

Non‐Nucleoside Reverse Transcriptase Inhibitors (NNRTIs): Past, Present, and Future

2004; Wiley; Volume: 1; Issue: 1 Linguagem: Inglês

10.1002/cbdv.200490012

ISSN

1612-1880

Autores

Erik De Clercq,

Tópico(s)

Pneumocystis jirovecii pneumonia detection and treatment

Resumo

Abstract Non‐nucleoside reverse transcriptase (RT) inhibitors (NNRTIs) have become an inherent ingredient of the drug combination schemes that are currently used in the treatment of human immunodeficiency virus type 1 (HIV‐1) infections. Starting from the 1‐[(2‐hydroxyethoxy)methyl]‐6‐(phenylsulfanyl)thymine (HEPT) and 4,5,6,7‐tetrahydroimidazo[4,5,1‐ jk ][1,4]benzodiazepin‐2(1 H )‐one and ‐thione (TIBO) derivatives, numerous classes of compounds have been described as NNRTIs. Only three compounds have so far been approved for clinical use: nevirapine, delavirdine, and efavirenz. NNRTIs are notorious for rapidly leading to virus‐drug resistance development, primarily based on the emergence of the K103N and Y181C mutations in the HIV‐1 RT. Newer NNRTIs, such as capravirine, dapivirine (TMC 125), and DPC 083, are resilient to these ‘NNRTI’ mutations, and, therefore, offer considerable promise as future anti‐HIV‐1 drugs. NNRTIs are targeted at a specific ‘pocket’ binding site within the HIV‐1 RT, that is distinct from, but both spatially and functionally related to, the catalytic site, where the nucleoside RT inhibitors (NRTIs) and nucleotide RT inhibitors (NtRTIs) interact. NNRTIs have acquired a definitive position, as part of a combination regimen with NRTIs and NtRTIs, in the first‐line treatment of HIV‐1 infections.

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