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Light‐Driven Activation of the [H 2 O(terpy)Mn III ‐μ‐(O 2 )‐Mn IV (terpy)OH 2 ] Unit in a Chromophore–Catalyst Complex

2011; Wiley; Volume: 6; Issue: 6 Linguagem: Inglês

10.1002/asia.201100030

1861-4728

Christian Herrero, Annamaria Quaranta, Stefano Protti, Winfried Leibl, A. William Rutherford, Dr Reza Fallahpour, Marie‐France Charlot, Ally Aukauloo,

CO2 Reduction Techniques and Catalysts

The Living Daylight: Ruthenium-based chromophores are employed as building blocks for a photo-active complex bearing a known water-oxidation catalytic system [(Terpy)2(MnIII-μ-(O2)-MnIV)]. Its activation by visible light has been studied by EPR spectroscopy. Detailed facts of importance to specialist readers are published as ”Supporting Information”. Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.