Image potential states in monolayer, bilayer, and trilayer epitaxial graphene studied with time- and angle-resolved two-photon photoemission spectroscopy

2014; American Physical Society; Volume: 89; Issue: 15 Linguagem: Inglês

10.1103/physrevb.89.155303

ISSN

1550-235X

Autores

Kazutoshi Takahashi, Masaki Imamura, Isamu Yamamoto, Junpei Azuma, Masao Kamada,

Tópico(s)

Quantum and electron transport phenomena

Resumo

Image potential states (IPSs) on monolayer, bilayer, and trilayer graphene epitaxially grown on SiC(0001) have been studied by time- and angle-resolved two-photon photoemission (2PPE) spectroscopy. The free-electron-like dispersions of even and odd symmetry IPSs with a quantum number of $n$ = 1${}^{+}$, 1${}^{\ensuremath{-}}$, 2, 3 were observed. All observed IPSs showed the dispersions with effective masses of ${m}^{*}=1.0\ifmmode\pm\else\textpm\fi{}0.1{m}_{e}$. The 2PPE intensity of the lowest IPS ($n$ = 1${}^{+}$) was attenuated with an increasing number of graphene layers. The time-resolved 2PPE measurements revealed that these IPSs have significantly shorter lifetimes, suggesting a coupling of IPSs with electronic states in the buffer layer and the SiC substrate.

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