Artigo Revisado por pares

Palladium-Catalyzed Synthesis of Butatrienes

2000; Oxford University Press; Volume: 29; Issue: 7 Linguagem: Inglês

10.1246/cl.2000.776

ISSN

1348-0715

Autores

Masamichi Ogasawara, Hisashi Ikeda, Kazunori Ohtsuki, Tamio Hayashi,

Tópico(s)

Catalytic C–H Functionalization Methods

Resumo

Abstract Palladium-catalyzed synthesis of functionalized butatrienes was achieved starting from 2-bromo-1-buten-3-yne derivatives and nucleophiles. The reaction proceeded under very mild conditions giving the products in moderate to good yields. The reactivity of the bromobutenyne substrates was highly dependent on substituents at 1-position. A subtle balance of nucleophilicity and basicity in the nucleophiles was also important for the success of the reactions.

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