Signatures of Bloch-Band Geometry on Excitons: Nonhydrogenic Spectra in Transition-Metal Dichalcogenides
2015; American Physical Society; Volume: 115; Issue: 16 Linguagem: Inglês
10.1103/physrevlett.115.166802
ISSN1092-0145
AutoresAjit Srivastava, Ataç İmamoğlu,
Tópico(s)Graphene research and applications
ResumoThe geometry of electronic bands in a solid can drastically alter single-particle charge and spin transport. We show here that collective optical excitations arising from Coulomb interactions also exhibit unique signatures of Berry curvature and quantum geometric tensor. A nonzero Berry curvature mixes and lifts the degeneracy of l≠0 states, leading to a time-reversal-symmetric analog of the orbital Zeeman effect. The quantum geometric tensor, on the other hand, leads to l-dependent shifts of exciton states that is analogous to the Lamb shift. Our results provide an explanation for the nonhydrogenic exciton spectrum recently calculated for transition-metal dichalcogenides. Numerically, we find a Berry curvature induced splitting of ∼10 meV between the 2px±i2py states of WSe2.
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