Artigo Revisado por pares

Hollow Ni/C microspheres derived from Ni-metal organic framework for electromagnetic wave absorption

2019; Elsevier BV; Volume: 383; Linguagem: Inglês

10.1016/j.cej.2019.123207

ISSN

1873-3212

Autores

Yun Qiu, Ying Lin, Haibo Yang, Lei Wang, Mengqi Wang, Bo Wen,

Tópico(s)

Metamaterials and Metasurfaces Applications

Resumo

Hollow nickel/carbon (Ni/C) microsphere was synthesized by in situ pyrolysis of the Ni-based trimellitic acid framework (Ni-MOF) at argon atmosphere. The morphology of Ni-MOF precursor can be easily controlled by adjusting the volume ratio of DMF and H2O in solvothermal process. When the volume ratio of DMF: H2O is 2: 1, hollow Ni-MOF microspheres can be obtained and the corresponding Ni/C composite exhibits extremely strong electromagnetic wave absorption. The maximum reflection loss is up to −57.25 dB with the matching thickness of only 1.8 mm, while the corresponding effective absorption bandwidth (reflection loss below −10 dB) achieves 5.1 GHz. The excellent electromagnetic wave absorbing capabilities is related to the hollow structure and the synergistic effect between carbon and nickel nanoparticles. This work confirms that the as-prepared Ni/C composite with superior electromagnetic wave absorption properties is a promising candidate for lightweight electromagnetic wave absorbing materials.

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