Artigo Revisado por pares

Titanium-supported W-containing PEO layers enriched with Mn or Zn in oxidative desulfurization and the zwitterionic liquid effect

2020; Elsevier BV; Volume: 393; Linguagem: Inglês

10.1016/j.surfcoat.2020.125746

ISSN

1879-3347

Autores

А. А. Брыжин, И. Г. Тарханова, M. G. Gantman, В. С. Руднев, M. S. Vasilyeva, I. V. Lukiyanchuk,

Tópico(s)

Catalytic Processes in Materials Science

Resumo

Titanium-supported oxide layers of W, W + Zn and W + Mn, formed by plasma electrolytic oxidation, were established to catalyze the peroxide oxidation of thiophene. The most active compositions based on Zn-W-containing PEO layers were also tested in the oxidation of a number of organosulfur compounds and diesel fuel desulfurization. Preliminary covering the samples by zwitterionic liquid (ZIL) made it possible to achieve residual sulfur content as low as 6 ppm. The change in the morphology and composition of samples with and without ZIL was studied during catalytic tests. It was found that ZIL reduces the etching of the sample surfaces when interacting with the reaction medium.

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