Artigo Acesso aberto Revisado por pares

Measurement of optical second-harmonic generation from an individual single-walled carbon nanotube

2013; IOP Publishing; Volume: 15; Issue: 8 Linguagem: Inglês

10.1088/1367-2630/15/8/083043

ISSN

1367-2630

Autores

Mikko J. Huttunen, Olli Herranen, Andreas Johansson, Hua Jiang, Prasantha R. Mudimela, Pasi Myllyperkiö, Godofredo Bautista, Albert G. Nasibulin, Esko I. Kauppinen, M. Ahlskog, Martti Kauranen, Mika Pettersson,

Tópico(s)

Photonic and Optical Devices

Resumo

We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the structural noncentrosymmetry, as required for SHG, arises from the non-zero chiral angle of the SWCNT. SHG thus has potential as a fast, non-destructive, and simple method for imaging of individual nanomolecules and for probing their chiral properties. Even more, it opens the possibility to optically determine the handedness of individual SWCNTs.

Referência(s)