Artigo Acesso aberto Revisado por pares

A dansyl-derivatized phytic acid analogue as a fluorescent substrate for phytases: experimental and computational approach

2021; Elsevier BV; Volume: 110; Linguagem: Inglês

10.1016/j.bioorg.2021.104810

ISSN

1090-2120

Autores

Christophe Dussouy, Éric Dubreucq, Patrick Chemardin, Véronique Perrier, Josiane Abadie, Hervé Quiquampoix, Claude Plassard, Jean‐Bernard Behr,

Tópico(s)

Oral and gingival health research

Resumo

A new myo-inositol pentakisphosphate was synthesized, which featured a dansyl group at position C-5.The fluorescent tag was removed from the inositol by a 6-atom spacer to prevent detrimental steric interactions in the catalytic site of phytases.The PEG linker was used in order to enhance hydrophilicity and biocompatibility of the new artificial substrate.Computational studies showed a favorable positioning in the catalytic site of phytases.Enzymatic assays demonstrated that the tethered myo-inositol was processed by two recombinant phytases Phy-A and Phy-C, classified

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