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Synthesis of 5‐Alkyl[3,4‐ c ]thienopyrrole‐4,6‐dione‐Based Polymers by Direct Heteroarylation

2011; Wiley; Volume: 124; Issue: 9 Linguagem: Inglês

10.1002/ange.201106411

1521-3757

Philippe Berrouard, Ahmed Najari, Agnieszka Proń, David Gendron, P. Morin, Jean‐Rémi Pouliot, Justine Veilleux, Mario Leclerc,

Sulfur-Based Synthesis Techniques

Angewandte ChemieVolume 124, Issue 9 p. 2110-2113 Zuschrift Synthesis of 5-Alkyl[3,4-c]thienopyrrole-4,6-dione-Based Polymers by Direct Heteroarylation† Philippe Berrouard, Philippe Berrouard Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDr. Ahmed Najari, Dr. Ahmed Najari Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDr. Agnieszka Pron, Dr. Agnieszka Pron Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDavid Gendron, David Gendron Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorPierre-Olivier Morin, Pierre-Olivier Morin Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorJean-Rémi Pouliot, Jean-Rémi Pouliot Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorJustine Veilleux, Justine Veilleux Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorProf. Dr. Mario Leclerc, Corresponding Author Prof. Dr. Mario Leclerc mario.leclerc@chm.ulaval.ca Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlDepartment of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this author Philippe Berrouard, Philippe Berrouard Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDr. Ahmed Najari, Dr. Ahmed Najari Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDr. Agnieszka Pron, Dr. Agnieszka Pron Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorDavid Gendron, David Gendron Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorPierre-Olivier Morin, Pierre-Olivier Morin Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorJean-Rémi Pouliot, Jean-Rémi Pouliot Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorJustine Veilleux, Justine Veilleux Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this authorProf. Dr. Mario Leclerc, Corresponding Author Prof. Dr. Mario Leclerc mario.leclerc@chm.ulaval.ca Department of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlDepartment of Chemistry, Université Laval, Quebec City, QC, G1V 0A6 (Canada) http://www.chm.ulaval.ca/poly_conducteurs/fr/marioleclerc.htmlSearch for more papers by this author First published: 11 November 2011 https://doi.org/10.1002/ange.201106411Citations: 31 † This work was supported by grants from the NSERC. The authors thank Professors F.-G. Fontaine and F. Ozawa for useful discussions and J. Delisle-Labrecque and W.-O. Caron for their technical assistance. Read the full textAboutPDF ToolsRequest permissionAdd to favorites ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onFacebookTwitterLinkedInRedditWechat Graphical Abstract Thiophen-Polymere durch Kreuzkupplung: Eine Polykondensation durch direkte Heteroarylierung führte nach wenigen Syntheseschritten zu Thienopyrroldion-haltigen Polymeren mit hohem Molekulargewicht (siehe Schema), wobei beeindruckende Ausbeuten bis 96 % erzielt wurden. Das neue Verfahren bietet eine Alternative zur üblichen Stille-Kupplung, ohne wie diese giftige Zinnverbindungen als Kupplungsprodukte zu erzeugen. Citing Literature Supporting Information Detailed facts of importance to specialist readers are published as "Supporting Information". Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Filename Description ange_201106411_sm_miscellaneous_information.pdf982.2 KB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume124, Issue9February 27, 2012Pages 2110-2113 This is the German version of Angewandte Chemie. Note for articles published since 1962: Do not cite this version alone. 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