Artigo Acesso aberto Revisado por pares

Methane Coupling over Magnesium Oxide: How Doping Can Work

2013; Wiley; Volume: 125; Issue: 43 Linguagem: Inglês

10.1002/ange.201305470

ISSN

1521-3757

Autores

Pierre Schwach, Marc‐Georg Willinger, Annette Trunschke, Robert Schlögl,

Tópico(s)

Mesoporous Materials and Catalysis

Resumo

Angewandte ChemieVolume 125, Issue 43 p. 11591-11594 Zuschrift Methane Coupling over Magnesium Oxide: How Doping Can Work† Pierre Schwach, Pierre Schwach Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorDr. Marc Georg Willinger, Dr. Marc Georg Willinger Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorDr. Annette Trunschke, Corresponding Author Dr. Annette Trunschke [email protected] Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplAbteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorProf. Dr. Robert Schlögl, Prof. Dr. Robert Schlögl Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this author Pierre Schwach, Pierre Schwach Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorDr. Marc Georg Willinger, Dr. Marc Georg Willinger Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorDr. Annette Trunschke, Corresponding Author Dr. Annette Trunschke [email protected] Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplAbteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this authorProf. Dr. Robert Schlögl, Prof. Dr. Robert Schlögl Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4–6, 12489 Berlin (Germany) http://www.fhi-berlin.mpg.de/acnew/welcome.eplSearch for more papers by this author First published: 17 September 2013 https://doi.org/10.1002/ange.201305470Citations: 14 † We thank M. Hashagen, F. Rybicki, Dr. F. Girgsdies, Dr. M. Eichelbaum, and Dr. O. Timpe for experimental support and scientific discussions. This work was conducted in the framework of the COE "UniCat" (www.unicat.tu-berlin.de) of the German Science Foundation. Read the full textAboutPDF ToolsRequest permissionAdd to favorites ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Graphical Abstract Elektronisches Doping: Die Dotierung von Magnesiumoxidkatalysatoren hat Auswirkungen auf die oxidative Kupplung von Methan. Hoch aktive Zentren entstehen durch eine Comodifizierung von MgO mit ppm-Mengen an Eisen und Gold. Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Filename Description ange_201305470_sm_miscellaneous_information.pdf5.4 MB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. References 1 1aH. Schwarz, Angew. Chem. 2011, 123, 10276; 10.1002/ange.201006424 Google ScholarAngew. Chem. Int. Ed. 2011, 50, 10096; 10.1002/anie.201006424 CASPubMedWeb of Science®Google Scholar 1bC. Hammond, S. Conrad, I. Hermans, ChemSusChem 2012, 5, 1668. 10.1002/cssc.201200299 CASPubMedWeb of Science®Google Scholar 2U. Zavyalova, M. Holena, R. Schlögl, M. Baerns, ChemCatChem 2011, 3, 1935. 10.1002/cctc.201100186 CASWeb of Science®Google Scholar 3T. Ito, T. Watanabe, T. Tashiro, K. Toi, J. Chem. Soc. Faraday Trans. 1 1989, 85, 2381. 10.1039/f19898502381 CASWeb of Science®Google Scholar 4 4aU. Zavyalova, M. Geske, R. Horn, G. Weinberg, W. Frandsen, M. Schuster, R. Schlögl, ChemCatChem 2011, 3, 949–959; 10.1002/cctc.201000098 CASWeb of Science®Google Scholar 4bU. Zavyalova, G. Weinberg, W. Frandsen, F. Girgsdies, T. Risse, K. P. Dinse, R. Schloegl, R. Horn, ChemCatChem 2011, 3, 1779–1788. 10.1002/cctc.201100146 CASWeb of Science®Google Scholar 5D. Beruto, A. W. Searcy, R. Botter, M. Giordani, J. Phys. Chem. 1993, 97, 9201–9205. 10.1021/j100138a022 CASWeb of Science®Google Scholar 6Y. Cui, N. Nilius, X. Shao, M. Baldofski, J. Sauer, H.-J. Freund, Angew. Chem.­ 2013, DOI: ; Angew. Chem. Int. Ed.­ 2013, DOI: . Google Scholar 7J. H. Lunsford, Angew. Chem. 1995, 107, 1059–1070; 10.1002/ange.19951070905 Google ScholarAngew. Chem. Int. Ed. Engl. 1995, 34, 970–980. 10.1002/anie.199509701 CASWeb of Science®Google Scholar 8J. S. J. Hargreaves, G. J. Hutchings, R. W. Joyner, C. J. Kiely, J. Catal. 1992, 135, 576–595. 10.1016/0021-9517(92)90055-M CASWeb of Science®Google Scholar 9K. Blick, T. D. Mitrelias, J. S. J. Hargreaves, G. J. Hutchings, R. W. Joyner, C. J. Kiely, F. E. Wagner, Catal. Lett. 1998, 50, 211–218. 10.1023/A:1019004110702 CASWeb of Science®Google Scholar 10G. Lehmann, Z. Phys. Chem. Neue Folge 1970, 72, 279–297. 10.1524/zpch.1970.72.4_6.279 CASWeb of Science®Google Scholar 11C. F. Bohren, D. R. Huffman, Absorption and Scattering of Light by Small Particles, Wiley, New York, 1983. Web of Science®Google Scholar 12K. C. Grabar, R. G. Freeman, M. B. Hommer, M. J. Natan, Anal. Chem. 1995, 67, 735–743. 10.1021/ac00100a008 CASWeb of Science®Google Scholar 13B. V. King, F. Freund, Phys. Rev. B 1984, 29, 5814–5824. 10.1103/PhysRevB.29.5814 CASWeb of Science®Google Scholar 14J. S. J. Hargreaves, G. J. Hutchings, R. W. Joyner, C. J. Kiely, Catal. Today 1992, 13, 401–407. 10.1016/0920-5861(92)80165-J CASWeb of Science®Google Scholar 15M. J. Hÿtch, E. Snoeck, R. Kilaas, Ultramicroscopy 1998, 74, 131. 10.1016/S0304-3991(98)00035-7 CASWeb of Science®Google Scholar 16P. Landon, P. J. Collier, A. J. Papworth, C. J. Kiely, G. J. Hutchings, Chem. Commun. 2002, 0, 2058. 10.1039/b205248m CASWeb of Science®Google Scholar 17G. J. Hutchings, Catal. Lett. 2001, 75, 1. 10.1023/A:1016784122682 CASWeb of Science®Google Scholar Citing Literature Volume125, Issue43October 18, 2013Pages 11591-11594 This is the German version of Angewandte Chemie. Note for articles published since 1962: Do not cite this version alone. Take me to the International Edition version with citable page numbers, DOI, and citation export. We apologize for the inconvenience. 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