Artigo Revisado por pares

Aryl CbH Activation by CuII To Form an Organometallic Aryl–CuIII Species: A Novel Twist on Copper Disproportionation This research was supported by MICYT of Spain through project PBQ2000-0548 and with the grant SGR-3102-UG-01 as well as the Distinction award from from CIRIT Generalitat de Catalunya (Spain). An FI doctoral grant from CIRIT to X.R. and financial support from the National Institutes of Health (USA; T.D.P.S. GM-50730; K.O.H. RR-01209) are also acknowledged. SSRL operations are …

2002; Wiley; Volume: 114; Issue: 16 Linguagem: Alemão

10.1002/1521-3757(20020816)114

ISSN

1521-3757

Autores

Xavi Ribas, Deanne A. Jackson, B. Donnadieu, José Mahía, Teodor Parella, Raà ⁄ l Xifra, Britt Hedman, Keith O. Hodgson, Antoni Llobet, T. Daniel P. Stack,

Tópico(s)

Cyclopropane Reaction Mechanisms

Resumo

Aus einfachen triazamakrocyclischen Liganden und Kupfer(II)-Salzen entstehen unter milden Bedingungen die Produkte einer intramolekularen Aryl-C-H-Aktivierung und Metall-Disproportionierung [Gl. (1)]. Die neuen metallorganischen CuIII-Komplexe sind unter protischen Bedingungen stabil.

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